The successful exfoliation of graphite initiated new science in any research field and is employing a huge number of scientists in the world investigating chemical, structural, mechanical and optoelectrical; properties of the atomic-thick sheets of graphene and graphene oxide.
Similarly to other carbon-based materials, graphene family have shown exceptional optical responses; and nowadays it is engineered to produce efficient photonic components. In this review we aim to summarize the main results in nonlinear optical response and fluorescence of graphene oxide; moreover, its laser printing is reviewed as a novel promising lithographic technique.
One of the most controversial phenomena in nonlinear dynamics is the reappearance of initial conditions. Celebrated as the Fermi-Pasta-Ulam-Tsingou problem, the attempt to understand how these recurrences form during the complex evolution that leads to equilibrium has deeply influenced the entire development of nonlinear science. The enigma is rendered even more intriguing by the fact that integrable models predict recurrence as exact solutions, but the difficulties involved in upholding integrability for a sufficiently long dynamic has not allowed a quantitative experimental validation. In natural processes, coupling with the environment rapidly leads to thermalization, and finding nonlinear multimodal systems presenting multiple returns is a long-standing open challenge. Here, we report the observation of more than three Fermi-Pasta-Ulam-Tsingou recurrences for nonlinear optical spatial waves and demonstrate the control of the recurrent behavior through the phase and amplitude of the initial field. The recurrence period and phase shift are found to be in remarkable agreement with the exact recurrent solution of the nonlinear Schrödinger equation, while the recurrent behavior disappears as integrability is lost. These results identify the origin of the recurrence in the integrability of the underlying dynamics and allow us to achieve one of the basic aspirations of nonlinear dynamics: the reconstruction, after several return cycles, of the exact initial condition of the system, ultimately proving that the complex evolution can be accurately predicted in experimental conditions.
Optical parametric oscillators are widely used as pulsed and continuous-wave tunable sources for innumerable applications, such as quantum technologies, imaging, and biophysics. A key drawback is material dispersion, which imposes a phase-matching condition that generally entails a complex design and setup, thus hindering tunability and miniaturization. Here we show that the burden of phase-matching is surprisingly absent in parametric micro-resonators utilizing mono-layer transition-metal dichalcogenides as quadratic nonlinear materials. By the exact solution of nonlinear Maxwell equations and first-principle calculations of the semiconductor nonlinear response, we devise a
novel kind of phase-matching-free miniaturized parametric oscillator operating at conventional pump intensities. We find that different two-dimensional semiconductors yield degenerate and non-degenerate emission at various spectral regions due to doubly resonant mode excitation, which can be tuned by varying the incidence angle of the external pump laser. In addition, we show that high-frequency electrical modulation can be achieved by doping via electrical gating, which can be used to efficiently shift the threshold for parametric oscillation. Our results pave the way for the realization of novel ultra-fast tunable micron-sized sources of entangled photons—a key device underpinning any quantum protocol. Highly miniaturized optical parametric oscillators may also be employed in lab-on-chip technologies for biophysics, detection of environmental pollution and security.
The intriguing connection between black holes’evaporation and physics of solitons is opening novel roads to finding observable phenomena. It is known from the inverse scattering transform that velocity is a fundamental parameter in solitons theory. Taking this into account, the study of Hawking radiation by a moving soliton gets a growing relevance. However, a theoretical context for the description of this phenomenon is still lacking. Here, we adopt a soliton geometrization technique to study the quantum emission of a moving soliton in a one-dimensional model. Representing a black hole by the one soliton solution of the Sine-Gordon equation, we consider Hawking emission spectra of a quantized massless scalarfield on the soliton-induced metric. We study the relation between the soliton velocity and the black hole temperature. Our results address a new scenario in the detection of new physics in the quantum gravity panorama.
The cascade of resonant topological structures with PT-symmetry breaking is shown to emit laser light with a frequency-comb spectrum. We consider optically active topological Aubry-Andr\’e-Harper lattices supporting edge-modes at regularly spaced frequencies. When the amplified resonances in the PT-broken regime match the edge modes of the topological gratings, we predict the emission of discrete laser lines. A proper design enables to engineer the spectral features for specific applications. The robustness of the topological protection makes the system very well suited for a novel generation of compact frequency comb emitters for spectroscopy, metrology, and quantum information.
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