In any form of wave propagation, strong spatiotemporal coupling appears when non-elementary, three-dimensional wave-packets are composed by superimposing pure plane waves, or spontaneously generated by light-matter interaction and nonlinear processes. Ultrashort pulses with orbital angular momentum (OAM), or ultrashort vortices, furnish a critical paradigm in which the analysis of the spatiotemporal coupling in the form of temporal-OAM coupling can be carried out accurately by analytical tools. By generalizing and unifying previously reported results, we show that universal and spatially heterogeneous space-time correlations occur in propagation-invariant temporal pulses carrying OAM. In regions with high intensity, the pulse duration has a lower bound fixed by the topological charge of the vortex and such that the duration must increase with the topological charge. In regions with low intensity in the vicinity of the vortex, a large blue-shift of the carrier oscillations and an increase of the number of them is predicted for strongly twisted beams. We think that these very general findings highlight the existence of a structural coupling between space and time, which is relevant at low photon numbers in quantum optics, and also in the highly nonlinear process as the high-harmonics generated with twisted beams. These results have also applications as multi-level classical and quantum free-space or satellite, communications, spectroscopy, and high-harmonic generation.
Miguel A. Porras and C. Conti in arXiv:1911.1222
Phys. Rev. A 101, 063803 (2020)
Terahertz absorption spectroscopy plays a key role in physical, chemical and biological systems as a powerful tool to identify molecular species through their rotational spectrum fingerprint. Owing to the sub-nanometer scale of molecules, radiation-matter coupling is typically dominated by dipolar interaction. Here we show that multipolar rotational spectroscopy of molecules in proximity of localized graphene structures can be accessed through the extraordinary enhancement of their multipolar transitions provided by terahertz plasmons. In particular, specializing our calculations to homonuclear diatomic molecules, we demonstrate that a micron-sized graphene ring with a nano-hole at the core combines a strong near-field enhancement and an inherently pronounced field localization enabling the enhancement of the dipole-forbidden terahertz absorption cross-section of H+2H2+ by 8 orders of magnitude. Our results shed light on the strong potential offered by nano-structured graphene as a robust and electrically tunable platform for multipolar terahertz absorption spectroscopy at the nanoscale.
A. Ciattoni, C. Conti, and A. Marini in Communication Physics
Laser & photonic reviews published the paper by Ciattoni et al. on the spin orbit coupling in graphene (arXiv version). The coupling of 2D electrons with OAM and Spin allows to control the state of nano-scale light beams, and is potentially useful for multilevel quantum gates.
We present a complete and consistent quantum theory of generalised X waves with orbital angular momentum in dispersive media. We show that the resulting quantised light pulses are affected by neither dispersion nor diffraction and are therefore resilient against external perturbations. The nonlinear interaction of quantised X waves in quadratic and Kerr nonlinear media is also presented and studied in detail.
M. Ornigotti, C. Conti, and A. Szameit, Journal of Optics 20 (2018) 065201
We develop a novel theoretical framework describing polariton-enhanced spin-orbit interaction of light on the surface of two-dimensional media. Starting from the integral formulation of electromagnetic scattering, we exploit the reduced dimensionality of the system to introduce a quantum-like formalism particularly suitable to fully take advantage of rotational invariance. Our description is closely related to that of a fictitious spin one quantum particle living in the atomically thin medium, whose orbital, spin and total angular momenta play a key role in the scattering process. Conservation of total angular momentum upon scattering enables to physically unveil the interaction between radiation and the two-dimensional material along with the detailed exchange processes among orbital and spin components. In addition, we specialize our model to doped extended graphene, finding such spin-orbit interaction to be dramatically enhanced by the excitation of surface plasmon polaritons propagating radially along the graphene sheet. We provide several examples of the enormous possibilities offered by plasmon-enhanced spin-orbit interaction of light including vortex generation, mixing, and engineering of tunable deep subwavelength arrays of optical traps in the near field. Our results hold great potential for the development of nano-scaled quantum active elements and logic gates for the manipulation of hyper-entangled photon states as well as for the design of artificial media imprinted by engineered photonic lattices tweezing cold atoms into the desired patterns.
A. Ciattoni, C. Rizza, H. W. H. Lee, C. Conti, A. Marini in ArXiv:1804.10533