Random media with tailored optical properties are attracting burgeoning interest for applications in imaging, biophysics, energy, nanomedicine, spectroscopy, cryptography and telecommunications. A key paradigm for devices based on this class of materials is the transmission matrix, the tensorial link between the input and the output signals, that describes in full their optical behavior. The transmission matrix has specific statistical properties, as the existence of lossless channels, that can be used to transmit information, and are determined by the disorder distribution. In nonlinear materials, these channels may be modulated and the transmission matrix tuned accordingly. Here we report the direct measurement of the nonlinear transmission matrix of complex materials, exploiting the strong optothermal nonlinearity of scattering Silica Aerogel (SA). We show that the dephasing effects due to nonlinearity are both controllable and reversible, opening the road to applications based on the nonlinear response of random media.
Many theories of quantum gravity, as string theory, loop quantum gravity, and doubly special relativity, predict the existence of a minimal length scale and outline the need to generalize the uncertainty principle. This generalized uncertainty principle relies on modified commutation relations that – if applied to the second quantization – imply an excess energy of the electromagnetic quanta with respect to ℏω. Here we show that this “dark energy of the photon” is amplified during nonlinear optical process. Therefore, if one accepts the minimal length scenario, one must expect to observe specific optical frequencies in optical harmonic generation by intense laser fields. Other processes as four-wave mixing and supercontinuum generation may also contain similar spectral features of quantum-gravity. Nonlinear optics may hence be helpful to falsify some of the most investigated approaches to the unification of quantum mechanics and general relativity.
Solitons and nonlinear waves emit resonant radiation in the presence of perturbations. This effect is relevant for nonlinear fiber optics, supercontinuum generation, rogue waves, and complex nonlinear dynamics. However, resonant radiation is narrowband, and the challenge is finding novel ways to generate and tailor broadband spectra. We theoretically predict that nonlinear self-accelerated pulses emit a novel form of synchrotron radiation that is extremely broadband and controllable. We develop an analytic theory and confirm the results by numerical analysis. This new form of supercontinuum generation can be highly engineered by shaping the trajectory of the nonlinear self-accelerated pulses. Our results may find applications in novel highly efficient classical and quantum sources for spectroscopy, biophysics, security, and metrology.
We present a complete and consistent quantum theory of generalised X waves with orbital angular momentum in dispersive media. We show that the resulting quantised light pulses are affected by neither dispersion nor diffraction and are therefore resilient against external perturbations. The nonlinear interaction of quantised X waves in quadratic and Kerr nonlinear media is also presented and studied in detail.